Journal
RSC ADVANCES
Volume 9, Issue 6, Pages 3429-3435Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ra10158b
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Funding
- National Natural Science Foundation of China [51502190]
- Program for the Outstanding Innovative Teams of Higher Learning Institutions of Shanxi
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In this paper, we report on highly efficient Mn4+-activated double perovskite Li3Mg2SbO6 (LMS) red-emitting phosphors. These LMS:Mn4+ phosphors can be efficiently excited over a broad wavelength band from 235 nm to 600 nm peaking at 344 nm and 469 nm, and exhibited an intense red emission band with a range from 600 nm to 800 nm centered around 651 nm. The optimal Mn4+ doping concentration of LMS:Mn4+ was 0.6 mol% and its internal quantum efficiency can reach as high as 83%. Besides, the thermal quenching effect on the optical property was also analyzed. Finally, a warm white light-emitting diode (WLED) lamp was fabricated by using a 454 nm InGaN blue LED chip combined with a blend of YAG: Ce3+ yellow phosphors and the as-prepared LMS: 0.6% Mn4+ red phosphors, which showed bright white light with CIE chromaticity coordinates (0.4093, 0.3725), correlated color temperature (CCT = 3254 K), color rendering index (CRI = 81) and luminous efficacy (LE = 87 lm/W).
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