4.7 Article

Biomass-burning smoke heights over the Amazon observed from space

Journal

ATMOSPHERIC CHEMISTRY AND PHYSICS
Volume 19, Issue 3, Pages 1685-1702

Publisher

COPERNICUS GESELLSCHAFT MBH
DOI: 10.5194/acp-19-1685-2019

Keywords

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Funding

  1. NASA [NNX14AN47G]
  2. UK EPSRC
  3. University of Sheffield Chemical and Biological Engineering Department
  4. Leverhulme Trust through a Leverhulme Research Centre Award [RC-2015-029]
  5. NASA Climate and Radiation Research and Analysis Programme
  6. NASA Earth Observing System MISR project
  7. NASA Atmospheric Composition Modeling and Analysis Programme
  8. University of Sheffield OnCampus Placement Programme
  9. NASA [678352, NNX14AN47G] Funding Source: Federal RePORTER

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We characterise the vertical distribution of biomass-burning emissions across the Amazon during the biomass-burning season (July-November) with an extensive climatology of smoke plumes derived from MISR and MODIS (2005-2012) and CALIOP (2006-2012) observations. Smoke plume heights exhibit substantial variability, spanning a few hundred metres up to 6 km above the terrain. However, the majority of the smoke is located at altitudes below 2.5 km. About 60% of smoke plumes are observed in drought years, 40 %-50 % at the peak month of the burning season (September) and 94% over tropical forest and savanna regions, with respect to the total number of smoke plume observations. At the time of the MISR observations (10:00-11:00 LT), the highest plumes are detected over grassland fires (with an averaged maximum plume height of similar to 1100 m) and the lowest plumes occur over tropical forest fires (similar to 800 m). A similar pattern is found later in the day (14:00-15:00 LT) with CALIOP, although at higher altitudes (2300 m grassland vs. 2000 m tropical forest), as CALIOP typically detects smoke at higher altitudes due to its later overpass time, associated with a deeper planetary boundary layer, possibly more energetic fires, and greater sensitivity to thin aerosol layers. On average, 3 %-20 % of the fires inject smoke into the free troposphere; this percentage tends to increase toward the end of the burning season (November: 15 %-40 %). We find a well-defined seasonal cycle between MISR plume heights, MODIS fire radiative power and atmospheric stability across the main biomes of the Amazon, with higher smoke plumes, more intense fires and reduced atmospheric stability conditions toward the end of the burning season. Lower smoke plume heights are detected during drought 800 m) compared to non-drought (1100 m) conditions, in particular over tropical forest and savanna fires. Drought conditions favour understory fires over tropical forest, which tend to produce smouldering combustion and low smoke injection heights. Droughts also seem to favour deeper boundary layers and the percentage of smoke plumes that reach the free troposphere is lower during these dry conditions. Consistent with previous studies, the MISR mid-visible aerosol optical depth demonstrates that smoke makes a significant contribution to the total aerosol loading over the Amazon, which in combination with lower injection heights in drought periods has important implications for air quality. This work highlights the importance of biome type, fire properties and atmospheric and drought conditions for plume dynamics and smoke loading. In addition, our study demonstrates the value of combining observations of MISR and CALIOP constraints on the vertical distribution of smoke from biomass burning over the Amazon.

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