Journal
MATERIALS RESEARCH BULLETIN
Volume 94, Issue -, Pages 291-297Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.materresbull.2017.06.023
Keywords
Z-scheme; Photocatalysis; Photocharge; (BiO)(2)CO3
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Funding
- Natural Science Foundation of China [51472005, 51272081]
- Natural Science Foundation of Educational Committee of Anhui Province [gxyqZD2016413, gxyqZD2016414]
- State Key Laboratory of Structural Chemistry [20160014]
- Innovation Team of Design and Application of Advanced Energetic Materials
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A novel Z-scheme AgliAg/I-(BiO)(2)CO3 composite was constructed through a two step in-situ transforming process. AgI nanoparticles were firstly generated on the surface of I-(BiO)(2)CO3 via ion-exchange step and then metallic Ag was formed by decomposing tiny of AgI in the photocatalytic process. Under visible light (lambda >400 nm), the as -prepared AgliAg/I-(BiO)(2)CO3 composite intensively enhanced activity for rhodamine B degradation with corresponding k(app) value 0.63h(-1) in comparison with the reference samples. By means of the metallic Ag bridge, AgliAg/I-(BiO)(2)CO3 displayed excellent separation efficiency of photocharges on the basis of a Z-scheme mechanism. Moreover, AgliAg/I-(BiO)(2)CO3 kept good stability under visible light. This study provides a universal way to in-situ construct highly efficient Z-scheme (BiO)(2)CO3-based photocatalytic system applied for eliminating contaminants in wastewater. (C) 2017 Elsevier Ltd. All rights reserved.
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