Journal
DALTON TRANSACTIONS
Volume 48, Issue 16, Pages 5144-5148Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9dt00645a
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Funding
- Natural Science Foundation of China [21501086, 21471009, 21671093]
- Shandong Provincial Natural Science Foundation [ZR2014BQ035, ZR2017MB052]
- Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry
- Liaocheng University
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A microporous metal-organic framework functionalized with in situ generated NHC-CuCl units (1) has been successfully synthesized from a novel imidazolium-containing ligand. In particular, the MOF 1 can catalyze -boration of ,-unsaturated carbonyl compounds, while the isoreticular version of 1 (1-im) modified with only imidazolium moiety cannot. This work demonstrates for the first time the heterogeneous catalysis of NHC-Cu(i)Cl within a MOF solid.
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