Journal
NEW JOURNAL OF CHEMISTRY
Volume 43, Issue 18, Pages 7130-7135Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8nj06146g
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Funding
- NSFC [51872161]
- Major Program of Shandong Provincial Natural Science Foundation [ZR2017ZB0316]
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Perovskite solar cells with a single light absorption heterojunction has demonstrated a power conversion efficiency of as high as 23.2% in the past few years. In this work, for the first time, we used quasi-spherical carbon quantum dots (CQDs)-doped PCBM film as the electron transporting layer of an inverted perovskite solar cell. The device structure is FTO/PEDOT: PSS/MAPbI(3)/PCBM: CQDs/BCP/Ag. The optimized PCE of 18.1% was achieved and a 13% enhancement was observed compared with those of pure PCBM-based devices. Various advanced characterizations including ultrafast spectroscopy, conductive atomic force microscopy, and electronic impedance spectroscopy elucidate that quasi-spherical CQD doping leads to enhanced electrical conductivity, electron mobility, and charge extraction efficiency. Moreover, we find that such CQD doping helps to prevent I- ions from undergoing interface diffusion and thus enhances the stability of solar cells.
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