Journal
CHEMICAL COMMUNICATIONS
Volume 55, Issue 29, Pages 4174-4177Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc01105f
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- U.S. National Science Foundation [CHE-1800471]
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Changing the solvent from H2O to D2O dramatically affects the branching of the initial excited electronic states in an alternating GC DNA duplex into two distinct decay channels. The slower, multisite PCET channel that deactivates more than half of all excited states in D2O becomes six times weaker in H2O.
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