Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 17, Issue 25, Pages 6122-6126Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9ob01086f
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Funding
- Anhui Provincial Natural Science Foundation [1708085MB29]
- National Natural Science Foundation of China [21871240, 21672198]
- Fundamental Research Funds for the Central Universities [WK2060190082]
- State Key Program of National Natural Science Foundation of China [21432009]
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A copper-catalyzed regioselective 1,4- and 1,6-conjugate addition of a silyl reagent to diendioates was established. Various 1,4- and 1,6-protosilylation products were obtained in good yields and with high regioselectivity via tuning the ligands used in the reactions. This protocol has provided a simple and efficient method for the synthesis of multisubstituted functionalized allylsilanes.
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