Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 139, Issue 40, Pages 13993-13996Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b07709
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Funding
- TAMU Chemistry Department
- Welch Foundation [A-1880]
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We present the first examples of CO2 electro-reduction catalysts that feature charged imidazolium groups in the secondary coordination sphere. The functionalized Lehn-type catalysts display significant differences in their redox properties and improved catalytic activities as compared to the conventional reference catalyst. Our results suggest that the incorporated imidazolium moieties do not solely function as a charged tag but also alter mechanistic aspects of catalysis.
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