Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 139, Issue 38, Pages 13300-13303Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b08347
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Funding
- National Natural Science Foundation of China [21522105]
- 1000 Young Talents Plan
- ShanghaiTech University
- National Postdoctoral Program for Innovative Talents [BX201600195, BX201700272]
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Mesoporous Zn4O(-COO)(6)-based metal organic frameworks (MOFs), including UMCM-1, MOF-205, MUF-7a, and the newly synthesized MOFs, termed ST-1, ST-2, ST-3, and ST-4 (ST = ShanghaiTech University), have been systematically investigated for ultra-high capacity methane storage. Exceptionally, ST-2 was found to have the highest deliverable capacity of 289 cm(3)srp/cm(3) (567 mg/g) at 298 K and 5-200 bar, which surpasses all previously reported records held by porous materials. We illustrate that the fine-tuned mesoporosity is critical in further improving the deliverable capacities at ultrahigh pressure.
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