Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 139, Issue 48, Pages 17293-17296Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b10519
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Funding
- NIH [GM-118641]
- LaMattina Graduate Fellowship
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The catalytic enantioselective conjunctive coupling of C(sp(3)) electrophiles can be accomplished with Ni catalysis. The enantioselectivity of the reaction is dependent on reaction mechanism with many substrates able to engage in an asymmetric process with Pybox-Ni complexes, whereas other substrates provide racemic product mixtures. The link between substrate structure and selectivity is addressed.
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