Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 139, Issue 42, Pages 14897-14900Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.7b09306
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Funding
- NIGMS [GM125206]
- Croucher Foundation, Hong Kong
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Visible light photoredox catalysis enables direct gamma- C(sp(3))-H alkylation of saturated aliphatic carbonyl compounds. Electron-deficient alkenes are used as the coupling partners in this reaction. Distinguished site selectivity is controlled by the predominant 1,5-hydrogen atom transfer of an amidyl radical generated in situ.
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