Journal
CHEMICAL SCIENCE
Volume 10, Issue 33, Pages 7728-7733Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9sc02616a
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Funding
- EPSRC [EP/P004997/1]
- European Research Council [758427]
- AstraZeneca
- Marie Curie Actions [791349]
- Marie Curie Actions (MSCA) [791349] Funding Source: Marie Curie Actions (MSCA)
- EPSRC [EP/P004997/1, 1735824] Funding Source: UKRI
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A divergent strategy for the remote arylation, vinylation and alkylation of nitriles is described. These processes proceed through the photoredox generation of a cyclic iminyl radical and its following ring-opening reaction. The distal nitrile radical is then engaged in nickel-based catalytic cycles to form C-C bonds with aryl bromides, alkynes and alkyl bromides.
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