Journal
JOURNAL OF RARE EARTHS
Volume 35, Issue 1, Pages 98-106Publisher
ELSEVIER
DOI: 10.1016/S1002-0721(16)60179-5
Keywords
PM2.5; rare earth elements; composition characteristics; distribution pattern; enrichment factor
Categories
Funding
- National Natural Science Foundation of China [21477042, 21377042]
- Natural Science Foundation of Fujian Province [2016J01065]
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Concentrations of sixteen rare earth elements (REEs) in PM2.5 and potential-source samples, collected in Nanchang city in mid-September 2013, were determined by inductively coupled plasma mass spectrometry (ICP-MS). The results showed that the concentrations of total REEs (Sigma REE) ranged from 78.76 to 1351 ng/mg. The order of REEs in PM2.5 samples showed the anthropogenic effects, Ce and Eu were affected more than the other REEs according to the enrichment factors. The results of chondrite-normalized REEs patterns and characteristic parameters showed evident light REEs fractionation, and positive anomalies of Ce and Eu in PM2.5. The other non-local pollution sources affected the PM2.5 samples, according to the triangular diagram of La, Ce and Sm compositions and plot of Sigma REE vs delta Eu. Moreover, plot of (La/Sm)(N) vs (Gd/Yb)(N) revealed the effects of local sources. In conclusion, the REEs in potential-source samples were close to the background of local soil, while the REEs in PM2.5 samples in Nanchang city were jointly affected by the investigated local sources and other non-local sources.
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