Journal
CHEMICAL COMMUNICATIONS
Volume 55, Issue 73, Pages 10884-10887Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc05522c
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Funding
- 1000 Plan Professorship for Young Talents, Hundred Talents Program of FuJian Province
- National Natural Science Foundation of China [21701175, 21703250, 21635002, 21705023]
- National Postdoctoral Program for Innovative Talents of China [BX201600164]
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The development of high-kinetic catalysts for the hydrogen evolution reaction (HER) in a neutral electrolyte is of great importance but unfortunately remains a challenge so far. Herein, we report hybrids with abundant Ru-S-Sb bonds and engineered ultrathin antimonene (Ru-S-Sb/antimonene) as highly kinetic, active, stable electrocatalysts for the HER in an aqueous neutral electrolyte. Experiments and density functional theory (DFT) calculations reveal that Ru-S-Sb bonds coupling with antimonene synergistically work to promote HER activity. The present study brings us one step closer to understand the structure-composition-property relationships and practical electrolytic H-2 production.
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