Journal
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS
Volume 111, Issue -, Pages 142-152Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.jpcs.2017.07.014
Keywords
Solid state reactions; Crystal structure; Magnetic and absorption measurements; Doped hexaferrites
Funding
- Ministry of Education and Science of the Russian Federation [K4-2015-040, K3-2016-019, K3-2017-028, K4-2017-041, 4.1346.2017/4.6]
- state order of the Russian Federation Government
- BRFBR [F17D-003]
- Act 211 of the Government of the Russian Federation [02.A03.21.0011]
- Russian Federation
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The BaFe12.5GaxO3.9 (x <= 1.2) hexaferrites were synthesized by the usual ceramic technology. It was been established that with the x increase the unit cell and magnetic parameters monotonically decrease. The frequency of natural ferromagnetic resonance firstly decreases from 49.6 GHz down to 49.1 GHz when x = 0.6 and then it increases up to 50.5 GHz. The line width monotonically increases from 3.5 GHz up to 5 GHz. The peak amplitude of resonant curve changes slightly with the exception for the x = 0.9 when it reaches -16 dB. The 1.3 GHz/kOe frequency shift in bias field is more intensive for small x = 0.3. The decreasing of the magnetic parameters is a result of the dilution of the Fe3+ - O2- - Fe3+ superexchange interactions. The behavior of the amplitude frequency characteristics is largely determined by the reduction of the uniaxial exchange anisotropy. The prospects of the Ga-substituted hexaferrites as a material effectively absorbing the high-frequency electromagnetic radiation are shown.
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