Journal
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 8, Issue 22, Pages 5487-5491Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.7b02060
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Funding
- Photon and Quantum Basic Research Coordinated Development Program from the Ministry of Education, Culture, Sports, Science and Technology, Japan
- European Research Council (ERC advanced grant WATER) [667205]
- Swedish Research Council
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We use resonant inelastic X-ray scattering (RIXS) to resolve vibrational losses corresponding to the OH stretch where the X-ray absorption process allows us to selectively probe different structural subensembles in liquid water. The results point to a unified interpretation of X-ray and vibrational spectroscopic data in line with a picture of two classes of structural environments in the liquid at ambient conditions with predominantly close-packed high-density liquid (HDL) and occasional local fluctuations into strongly tetrahedral low-density liquid (LDL).
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