Journal
CHEMICAL COMMUNICATIONS
Volume 55, Issue 84, Pages 12635-12638Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc06763a
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Funding
- FCT/MEC [UID/CTM/50011/2019]
- FEDER through COMPETE 2020 [022161]
- FEDER through POCI [022161]
- FEDER through PORL [022161]
- FCT through PIDDAC [022161]
- FCT [PD/BD/142849/2018, PD/00065/2013, 007630 UID/QUI/00313/2013, UID/QUI/00100/2019]
- COMPETE2020-UE
- Fundação para a Ciência e a Tecnologia [PD/BD/142849/2018] Funding Source: FCT
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Two-dimensional H-1-P-31 heteronuclear correlation NMR of trimethylphosphine oxide (TMPO) adsorbed in zeolites, in tandem with DFT calculations, challenges previous one-dimensional P-31 NMR assignments, enabling the unambiguous discrimination of Bronsted and Lewis acid sites, extending the understanding of TMPO:Bronsted complexes formed with distinct stoichiometries at the HZSM-5 zeolite surface, and the proton-transfer mechanism.
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