Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 82, Issue 12, Pages 6163-6171Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.7b00752
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Funding
- National Natural Science Foundation of China [21002076, 21441007]
- Graduate Education Innovation Fund of the Wuhan Institute of Technology [CX2016162, CX2016167]
- Project of the Natural Science Foundation of Hunan Province [2016JJ4072]
- Scientific Research Fund of the Hunan Provincial Education Department [16A165]
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An efficient copper-catalyzed C-N bond formation by N-H/C-H cross-dehydrogenative coupling (CDC) between NH-1,2,3-triazoles and N,N-dialkylamides has been developed. The method provided N-amidoalkylated 1,2,3-triazoles with moderate to high yields, and the reactions showed high N-2-selectivities when 4,5-disubstituted NH-1,2,3-triazoles served as the substrates.
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