Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 82, Issue 15, Pages 8067-8071Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.7b01328
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- Ministry of Science and Technology, Taiwan [103-2120-M-009-003-CCI]
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Here, we report the synthesis and characterization of a series of contorted, yet noncentrosymmetrical, polycyclic aromatic hydrocarbons with a pentabenzo-fused coronene as the core framework. The parent pentabenzo[a,d,g,j,m]coronene (PBC) compound is shown to exhibit a shifted and rotated type of pi-pi stacking interactions, which render this series a semiconducting material. Single-crystal-based field-effect transistor devices of PBC exhibited efficient charge transport behavior, giving a p-channel field-effect mobility of 0:42 cm(2) V(-1)s(-1) and an on/off ratio of 10(5).
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