Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 82, Issue 8, Pages 4113-4120Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.6b03095
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Funding
- National Natural Science Foundation of China [21471108, 21373142, 21531006]
- Natural Science Foundation of Jiangsu Province [BK20161276]
- State Key Laboratory of Organometallic Chemistry of Shanghai Institute of Organic Chemistry [2015kf-07]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- Soochow Scholar Program of Soochow University
- State and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials
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RuCl3 efficiently catalyzes the alkylation of methylquinolines, methylpyridines, 2-methyl-benzooxazoles, and 2-methyl-quinoxa-lines with alkyl- or aryl-alcohols as alkylating agents. This synthetically useful and atom economical transformationdoes not require additional ligands.The mechanistic study indicated the alkylation reaction underwent a stepwise transfer hydrogenation, aldol condensation, and hydrogenation reaction pathway.
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