Journal
ENERGYCHEM
Volume 1, Issue 3, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.enchem.2019.100015
Keywords
Dye-sensitized photoelectrochemical cells; Water splitting; Solar fuel; Hydrogen production
Categories
Funding
- National Natural Science Foundation of China [21971064, 21772040, 21572062]
- Shanghai Municipal Science and Technology Major Project [2018SHZDZX03]
- Fundamental Research Funds for the Central Universities [222201717003, 50321101918001]
- Programme of Introducing Talents of Discipline to Universities [B16017]
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Dye-sensitized photoelectrochemical cells (DSPECs) that can drive water splitting to generate solar fuel through the absorption of sun light, has attracted growing interest in the past decade. DSPECs consists of wide band gap nanoparticle metal oxide semiconductors and chromophore-catalyst assemblies, aiming to drive the two half reactions of water splitting at physically separated two compartments. Herein, we review the recent developments in the design of dye-sensitized photoanodes, photocathodes and tandem cells for water splitting, highlighting the strategies of sensitizers and catalysts assembly, core-shell electrodes fabrication and constructions of tandem device to enhance the efficiency and stability of water splitting DSPECs. Future challenges towards the development of more efficient and stable DSPECs are addressed in the end.
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