Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 6, Issue 21, Pages 3688-3692Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9qo00830f
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Funding
- National Natural Science Foundation of China [NSFC21572272]
- Innovation Team of the Double-First Class Disciplines [CPU2018GY04, CPU2018GY35]
- Foundation of the Open Project of State Key Laboratory of Natural Medicines [SKLNMZZCX201818]
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A rhodium(iii)-catalyzed C-H activation/annulation of salicylaldehydes with sulfoxonium ylides has been developed for the formation of 2-substituted chromones in good yields with broad functional group tolerance. The utility of this strategy was showcased by the late-stage modification of some biologically active molecules. Moreover, structurally diverse 2,3-disubstituted chromones were also constructed by the C3 C-H functionalization reactions.
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