Journal
ACS APPLIED POLYMER MATERIALS
Volume 1, Issue 11, Pages 2981-2989Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsapm.9b00686
Keywords
haze cellulose nanopaper; self-absorption; PMMA/AVB particle; range-broadening ultraviolet-blocking; hydrophobicity
Funding
- National Natural Science Foundation of China [21703131, 31370578]
- Doctoral Scientific Research Foundation of Shaanxi University of Science Technology [2016BJ-40]
- State Key Laboratory of Pulp and Paper Engineering [201821]
- Shaanxi Provincial Department of Education [18JK0122]
- Chinese Postdoctoral Science Foundation [2018M643707]
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Cellulose nanopaper-based materials with recyclability and excellent optical properties have recently received increasing attention. A series of lignin-containing (17.2, 14.7, 7.3, 4.9, and 1.3% by wt) pristine nanopapers (LNPs) were obtained through self-absorption of poly(methyl methacrylate) (PMMA)/avobenzone (AVB) to produce cellulose nanopapers (LPANPs) with range-broadening and ultraviolet (UV) blocking extending from UVB (290-320 nm) to UVA (320-400 nm). SEM results indicated that PMMA/AVB presented a microspherical morphology (150-600 nm) on LPANP surfaces. LPANP exhibited high optical transparency (>95% in the visible region) and high haze (>77%), with good wet mechanical properties (107.5 MPa) and thermal stability. In addition, LPANP hydrophobic properties were significantly improved after PMMA/AVB particle absorption, achieving conversion from hydrophilicity to hydrophobicity. Consequently, with the properties of water resistance, optical haze, and range-broadening UV-blocking, these LPANP presented potential applications in the field of optoelectronic devices, such as in UV-blocking, supercapacitors, and electronic device substrates.
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