Journal
ACS APPLIED POLYMER MATERIALS
Volume 1, Issue 11, Pages 2819-2825Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsapm.9b00269
Keywords
underwater superpolymphobicity; microfluidic channels; microfluidic systems; femtosecond laser; PDMS
Funding
- Bill & Melinda Gates Foundation [OPP1119542]
- National Key Research and Development Program of China [2017YFB1104700]
- National Science Foundation of China [51335008, 61875158, 61805192]
- China Postdoctoral Science Foundation [2016M600786]
- Fundamental Research Funds for the Central Universities [xzy012019042]
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A strategy is proposed here to fabricate microfluidic channels based on underwater superpolymphobic microgrooves with nanoscale rough surface structure on glass surface produced by femtosecond (fs) laser processing. The fs laser-induced micro/nanostructure on glass surface can repel liquid polydimethylsiloxane (PDMS) underwater, with the contact angle (CA) of 155.5 +/- 2.5 degrees and CA hysteresis of 2.7 +/- 1.5 degrees to a liquid PDMS droplet. Such a phenomenon is defined as the underwater superpolymphobicity. Microchannels as well as microfluidic systems are easily prepared and formed between the underwater superpolymphobic microgroove-textured glass substrate and the cured PDMS layer. Because the tracks of the laser scanning lines are programmable, arbitrary-shaped microchannels and complex microfluidic systems can be potentially designed and prepared through fs laser direct writing technology. The concept of underwater superpolymphobicity presented here offers us a new strategy for selectively avoiding the adhesion at the polymer/substrate interface and controlling the shape of cured polymers; none of these applications can find analogues in previously reported superwetting materials.
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