Journal
CHEMICAL COMMUNICATIONS
Volume 55, Issue 91, Pages 13765-13768Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc06170c
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Funding
- Japan Science and Technology Agency (JST) CREST [JPMJCR15P1]
- Japan Society for the Promotion of Science (JSPS) Kakenhi [18H02055]
- China Scholarship Council [201708050022]
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A hot-carrier-driven photocatalytic system was established by incorporating noble metals (Rh, Pd, Ru, and Pt) in a mesoporous silica (MCM-41) for the partial oxidation of methane (POM) under ultraviolet (UV) irradiation. The Rh/MCM photocatalyst initiated POM at a mild operating temperature of 423 K with syngas generation. The reaction was identified as a synergistic photothermal and photochemical process.
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