Journal
CHEMICAL COMMUNICATIONS
Volume 55, Issue 98, Pages 14729-14732Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc05233j
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Funding
- National Natural Science Foundation of China [81602977]
- CAMS Basic and Innovation Fund for Medical Sciences [2019-RC-HL-010, 2017-I2M-1-013, 2016-I2M-1-012]
- National Major Scientific and Technological Special Project [2015ZX 09501005]
- Science and Technology Development Project of Jilin Province of China [20190304050YY, 2017QNRC001]
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A palladium-promoted oxidative annulation reaction for the synthesis of structurally diverse naphthoquinone-containing heterocycles has been developed, providing switchable access to 1,2-naphthofuroquinones and densely functionalized cyclobutene-fused 1,4-naphthofuroquinones by selective enol/enolate-directed processes. The synthetic application was extended by late-stage functionalization of an anti-HIV drug. The practical value of 1,2-naphthofuroquinone synthesis was highlighted in endothelial protective lead compound development.
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