Journal
CHINESE JOURNAL OF ORGANIC CHEMISTRY
Volume 39, Issue 11, Pages 3065-3083Publisher
SCIENCE PRESS
DOI: 10.6023/cjoc201905016
Keywords
cross dehydrogenation coupling; visible-light-induced; transition metal-free; functionalization
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Funding
- Natural Science Foundation of Zhejiang Province [LY17C140003]
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The cross dehydrogenation coupling reaction realizes direct coupling of two different X-H bonds to form a new chemical bond, thus featuring excellent step and atom economy. The traditional cross dehydrogenation coupling reaction was usually catalyzed by transition metal, which had the problems of expensive catalyst and serious pollution. Visible light-induced electron transfer is also an effective way to realize direct functionalization of X-H bonds. Visible-light-induced cross dehydrogenation coupling reaction under transition metal-free conditions is widely concerned due to the advantages of cleanliness, safety as well as high step and atom economy. Classified by the type of bonding, the research progress of these reactions is reviewed, and their future outlook is also discussed.
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