Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 6, Issue 24, Pages 3956-3960Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9qo01011d
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Funding
- National Natural Science Foundation of China [21532006, 21690074]
- Chinese Academy of Sciences [XDB17020300]
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Kinetic resolution of [2.2]paracyclophane aldimines was achieved through palladium-catalyzed enantioselective arylation with arylboronic acids. The catalytic process provided reliable access to enantiopure paracyclophane derivatives with planar and central chirality as well as the recovered chiral aldimines with a selectivity factor up to 368. Furthermore, the synthetic utility of the [2.2]paracyclophane aldimines has been demonstrated by converting them into useful chiral building blocks.
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