Journal
JOURNAL OF MATERIALS SCIENCE
Volume 52, Issue 14, Pages 8421-8431Publisher
SPRINGER
DOI: 10.1007/s10853-017-1082-x
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Funding
- National Natural Science Foundation of China [61504076, 21574076, U1510121]
- National Natural Science Foundation of Shanxi Province [2015021129, 2014011016-1]
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Honeycomb-like polypyrrole/multi-wall carbon nanotube (PPy/MWCNT) film demonstrates as an efficient and semitransparent counter electrode (CE) in bifacial dye-sensitized solar cell (DSSC), which is first fabricated on fluorine-doped tin oxide glass by a facile method using a sacrificial template of poly(methyl methacrylate) (PMMA). The results from ultraviolet-visible spectrophotometer and cyclic voltammetry measurements testify that the honeycomb-like PPy/MWCNT film possesses high transparency for the backside illumination and wonderful electrocatalytic activity for the reduction of triiodide (I-3 (-)) to iodide (I-) in the bifacial DSSC. Electrochemical impedance spectroscopy results indicate that the honeycomb-like nanostructure combining with the MWCNT decreases the resistance of the PPy/MWCNT film for the transfer of electrons from the external circuit back to the redox electrolyte. The bifacial DSSC based on the honeycomb-like PPy/MWCNT CE achieves 7.07 and 4.11% of the front and rear efficiencies, respectively, which are higher than those of the bifacial DSSC based on the flat PPy CE (5.78 and 3.07%, respectively).
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