Journal
ACS APPLIED NANO MATERIALS
Volume 2, Issue 10, Pages 6763-6768Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsanm.9b01702
Keywords
nitrogen-rich; nanoparticle; chemoselectivity; hydrogenation; quinolines
Funding
- National Natural Science Foundation of China [NSFC: 21401004, 21973029, 21571092]
- Natural Science Foundation of Anhui Province [1508085QB36]
- Doctoral Scientic Research Foundation [070138]
- Open Foundation of Anhui Laboratory of Molecular-based Materials [fzj19005]
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Synergistic effects of multimetallic catalysts play a crucial role in the field of heterogeneous catalysis, especially in the oxidation and reduction of functional groups. Hence, how to design a multimetallic catalyst with high catalysis performance attracts the attention of scientists. Herein, we have designed and synthesized a cobalt nickel bimetallic catalyst step by step. More interestingly, the cobalt nickel nanoparticles were encapsulated in N-doped hollow porous carbon (HPC), on which were grown many carbon tubes. The optimized nanoparticle as a hydrogenation catalyst exhibits superior performance in the selective reduction of quinoline at ambient temperature, due to its advantage of dispersing uniform bimetal nanoparticles and N-doped active sites.
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