Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 7, Issue 1, Pages 126-130Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9qo01229j
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Funding
- National Natural Sciences Foundation of China [21871044, 21472017]
- Natural Sciences Foundation of Jilin Province [20190201073JC]
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A novel rhodium-catalyzed homodimerization-cyclization reaction of two vinyl isocyanides has been developed for the first time. In this reaction, the highly reactive 1,4-diazabutatriene intermediates generated by the homodimerization of two vinyl isocyanides could undergo a novel type of intramolecular tandem cyclization and provides a new and highly efficient method for the construction of 2-(isoquinolin-1-yl)oxazoles by formation of three new bonds and two rings from readily available acyclic starting materials in a single step.
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