Journal
CHEMICAL SCIENCE
Volume 11, Issue 6, Pages 1538-1541Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9sc05757a
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Funding
- Japan Society of the Promotion of Science (JSPS) from the Ministry of Education, Culture, Sports, Science and Technology, Japan [JP18H02032, JP19K22200]
- Strategic International Collaborative Research Program (SICORP) from the Japan Science and Technology, Japan
- Adaptable and Seamless Technology Transfer Program through Target-driven R&D (A-STEP) from the Japan Science and Technology, Japan
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We studied the relationship between proton conductivity and the terahertz-regime vibrations of two-dimensional MOFs. The results of spectroscopy studies clarified the essential role played by the collective motions in the terahertz region in 2D layers for efficient H+ conduction. Ab initio calculations suggested the collective motion to be predominantly determined by the valence electronic structure, depending on the identity of the metal ion.
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