Journal
JOURNAL OF CHEMICAL PHYSICS
Volume 146, Issue 9, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.4972073
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Funding
- Israel Science Foundation [1666/14]
- German Israel Foundation [1146-73.14]
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Due to bandwidth limitations of state of the art electronics, the transient transport properties of molecular junctions are experimentally a terra incognita, which can only be explored if novel picosecond current-probing techniques are developed. Here we demonstrate one such approach: the laser pulse pair sequence scheme. The method is used to monitor in picosecond resolution the oxidation state of a redox molecule, 6-ferrocenyl-1-hexanethiol, within a junction and to quantify its redox rate constant, which is found to be (80 ps)(-1). Published by AIP Publishing.
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