4.7 Article

Synthesis and post-synthetic modification of amine-, alkyne-, azide- and nitro-functionalized metal-organic frameworks based on DUT-5

Journal

DALTON TRANSACTIONS
Volume 44, Issue 38, Pages 16802-16809

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c5dt02276b

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Funding

  1. DFG
  2. Helmholtz Research School Energy-related Catalysis
  3. FCI

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Functionalized 4,4'-biphenyldicarboxylic acid molecules with additional amine, alkyne, azide or nitro groups were prepared and applied in the synthesis of novel metal-organic frameworks and mixed-linker metal-organic frameworks isoreticular to DUT-5. The properties of the frameworks could be tuned by varying the number of functional groups in the materials and the amine groups were employed in post-synthetic modification reactions without changing the framework structure or significantly decreasing the porosity of the materials.

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