Journal
MATTER
Volume 2, Issue 4, Pages 805-815Publisher
CELL PRESS
DOI: 10.1016/j.matt.2020.02.003
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Funding
- National Key R&D Program of China [2018YFB0104300]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA22010600]
- National Natural Science Foundation for Distinguished Young Scholars of China [51625204]
- National Natural Science Foundation of China [U1706229]
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Higher energy storage in the limited space of lithium batteries always brings more safety hazards. To address this issue, the utilization of solid electrolyte to replace the liquid one is a promising strategy. However, the sluggish charge transfer and poor interfacial compatibility between solid electrodes and solid electrolyte severely hinder the performance of high-energy-density solid-state lithium batteries. Thus, in this Perspective, the bottlenecks and the related solutions regarding organic/inorganic composite electrolyte, lithium-metal anode, and high-voltage cathode are focused on, and compatible interface engineering is presented. Aiming at the commercialization of high-energy-density solid-state lithium-metal batteries, possible strategies on tackling the remaining challenges of manufacturing scale are also highlighted.
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