Journal
DALTON TRANSACTIONS
Volume 44, Issue 6, Pages 2893-2896Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4dt03594a
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Funding
- 973 program [2012CB821705, 2011CB932504]
- NSFC [21425102, 21221001]
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A special organic ligand, 4-carboxypyrazole (4-cpz),is chosen to synthesize a highly stable metal-organic framework (MOF) for selective sorption of light hydrocarbons. The new MOF, (H3O)[Zn-3(OH)(4-cpz)(3)]center dot 2(DEF)center dot H2O (FIR-51, DEF = N, N-diethylformamide), was synthesized solvothermally and shows unusual chemical stability. This compound exhibits high storage capacity for light hydrocarbons and high selectivity for C3 and C2 over methane at 273 and 294 K.
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