Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 26, Pages 3761-3764Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cc09475j
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Funding
- NSF [CHE-1465188, DGE 1752814]
- U.S. DOE Integrated University Program
- NIH [S10OD023532]
- Office of Science, Office of Basic Energy Sciences, of the U.S. DOE [DE-AC02-05CH11231]
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We report a series of beta-diketiminate (BDI) complexes in which tautomeric rhenium(iii) hydride and rhenium(i) protio-BDI species readily interconvert between the solid and solution states. This phenomenon, which is only operative when an electron-accepting ligand is bound to rhenium, was investigated by a combination of experimental and computational methods.
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