Journal
DALTON TRANSACTIONS
Volume 49, Issue 11, Pages 3388-3392Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0dt00432d
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Funding
- Natural Science Foundation of Hebei Province [E2019201049]
- National Natural Science Foundation of China [51872324, 21763026]
- Advanced Talents Incubation Program of Hebei University [801260201293]
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A new family of non-centrosymmetric (NCS) compounds Sr(6)A(4)M(4)S(16) (A = Ag, Cu; M = Ge, Sn) with mixed tetrahedral anionic ligands (AS(4) and MS4) was successfully synthesized and characterized for the first time. All of the compounds exhibit excellent performances as promising infrared nonlinear optical (IR NLO) materials, with large NLO responses (1.1-2.0 x benchmark AgGaS2), high laser damage thresholds (2.0-4.5 x AgGaS2) and wide IR transmission ranges, and are nonhygroscopic. Moreover, their property modulation by the combination of different anionic groups was also discussed.
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