Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 32, Pages 4400-4403Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc01770a
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Funding
- National Science Foundation [DMR-1644779, CHE-1058077, CHE-1900491]
- NIH-MBRS RISE program [5R25GEMO71381]
- State of Florida
- U.S. Department of Energy, Office of Energy Sciences Materials Sciences Division [DE-AC0205CH11231]
- University of Idaho
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Coordination of 1-isopropyl-3,5-dipyridyl-6-oxoverdazyl to cobalt results in a dication best described in the solid state as a high spin cobalt(II) ion coordinated to two radical ligands with an S = 3/2 ground state. On dissolution in acetonitrile, the cobalt(II) form equilibrates with a cobalt(III) valence tautomer with an S = 1/2 ground state.
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