Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 32, Pages 4396-4399Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc01345e
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Funding
- National Natural Science Foundation of China [21606108, 21576119, 21878127]
- Neimenggu Key Science and Technology Plan of 2019
- Ordos Key Science and Technology Plan of 2019
- Fundamental Research Funds for the Central Universities [JUSRP51720B]
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The different chemical states and locations of Ni species in HZSM-5 result in different directions of CH4 reaction. Supported Ni clusters caused complete CH4 decomposition, while Ni-exchanged sites anchored at Bronsted acid sites, can appropriately activate CH4 into CHx species which are important precursors to produce aromatics. This study suggests a catalyst construction strategy for selective conversion of CH4 towards value-added chemicals by placing active metal at specific sites.
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