4.6 Article

Coherent control of 40-THz optical phonons in diamond using femtosecond optical pulses

Journal

PHYSICAL REVIEW B
Volume 101, Issue 17, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.101.174301

Keywords

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Funding

  1. JSPS KAKENHI, Collaborative Research Project of Laboratory for Materials and Structures, Institute of Innovative Research, Tokyo Institute of Technology [15K13377, 17K19051, 17H02797, 19K03696, 19K22141]
  2. Grants-in-Aid for Scientific Research [19K22141, 19K03696, 17H02797, 15K13377, 17K19051] Funding Source: KAKEN

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A theory of the coherent control of optical phonons by double-pulse excitation was modified for the calculation of a large detuning case such as diamond; we calculated the amplitude of the optical phonons without using a rotating-wave approximation. Additionally, we took the frequency chirping and non-Gaussian pulse shape into consideration. The coherent control of the amplitude of 40 THz optical phonons in diamond was demonstrated by using a pair of infrared pulses at a pump-pump delay between -10 and 120 fs, and analyzed by using the modified theory.

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