Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 43, Pages 5791-5794Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc01131b
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Funding
- KU Leuven [C14/19/78]
- SCDD, Govt. of Kerala, India
- Research Foundation - Flanders (FWO) [1SC4719N]
- China Scholarship Council (CSC)
- KU Leuven Internal Funds
- Hercules Foundation [AKUL/09/0035]
- Hercules Foundation of the Flemish Government [20100225-7]
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New easily functionalisable and highly fluorescent BOPAHY chromophores are synthesised via a one-pot two-step reaction starting from commercially available pyrrole-2-carbaldehydes and respective acyl hydrazides in the presence of BF3 center dot OEt2. Most importantly, all BOPAHY dyes show excellent photophysical properties with quantum yields up to 0.92. Steady-state spectroscopy and quantum chemical calculations provide a first insight into these promising properties.
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