4.7 Article

A stabilized PEO-based solid electrolyte via a facile interfacial engineering method for a high voltage solid-state lithium metal battery

Journal

CHEMICAL COMMUNICATIONS
Volume 56, Issue 42, Pages 5633-5636

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc01829e

Keywords

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Funding

  1. National Key R&D Program of China [2018YFB0104400]
  2. National Natural Science Foundation of China [51822211, U1932220, U19A2018]

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A facile interfacial engineering method via in situ electro-deposition was developed to stabilize the PEO-based solid electrolyte in high voltage solid-state lithium metal batteries (Li/PEO-LiTFSI/LiNi0.5Co0.2Mn0.3O2), which demonstrate a superior capacity retention of 72.3% after 200 cycles in 3.0-4.2 V. The critical factors for the interfacial engineering method were also demonstrated in this study.

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