Journal
MATERIALS CHEMISTRY FRONTIERS
Volume 4, Issue 7, Pages 2018-2022Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0qm00190b
Keywords
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Funding
- European Union's Horizon 2020 research and innovation programme under the Marie Skodowska Curie grant [838009, 838885]
- Marie Skodowska-Curie Individual Fellowship
- National Postdoctoral Program for Innovative Talents [BX201700164]
- Jiangsu Planned Projects for Postdoctoral Research Funds [2018K011A]
- Leverhulme Trust [RPG-2016047]
- EPSRC [EP/P010482/1]
- Fonds de la Recherche Scientifiques de Belgique (F. R. S.-FNRS) [2.5020.11]
- EPSRC [EP/P010482/1] Funding Source: UKRI
- Marie Curie Actions (MSCA) [838009] Funding Source: Marie Curie Actions (MSCA)
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The development of multiple resonance thermally activated delayed fluorescence (MR-TADF) materials possessing narrow emission spectra has attracted significant attention as emitters for high colour purity organic light emitting diodes (OLEDs). In this work, a simple design strategy is introduced to construct an MR-TADF emitter,DDiKTa, through dimerization of the known MR-TADF emitterDiKTa. This design permits concentration quenching to be largely suppressed, which is a known weakness of previously reported MR-TADF emitters. OLEDs based onDDiKTashow an EQE(max)of 19% at a doping concentration of 9 wt%. The electroluminescence spectrum is red-shifted into the green, producing a rare example of a green-emitting MR-TADF OLED.
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