Journal
DALTON TRANSACTIONS
Volume 49, Issue 22, Pages 7304-7308Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0dt01340d
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Funding
- National Natural Science Foundation of China [21731002, 21871172, 21801095]
- Major Program of Guangdong Basic and Applied Research [2019B030302009]
- Fundamental Research Funds for the Central Universities [21619405]
- Jinan University
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Two mixed-valence Cu-II/Cu(I)and two heterometallic Cu-II/Ag(I)metallocycles have been synthesized by the assembly of designed metalloligands and Cu-I/Ag(I)ions, respectively. The Cu-II/Cu(I)metallocycle can catalyze the oxidation of alcohols to aldehydes mediated by a co-catalyst, TEMPO (2,2,6,6-tetramethylpiperdine-1-oxyl), with ambient air as an oxidant, while the Cu-II/Ag(I)metallocycle has no catalytic effect.
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