Journal
NANOSCALE
Volume 12, Issue 25, Pages 13398-13406Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0nr02290j
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Funding
- Science and Technology Planning Project of Guangdong Province, China [2017B090916002]
- National Natural Science Foundation of China [51922042, 51872098]
- Guangdong Natural Science Funds for Distinguished Young Scholar [2016A030306010]
- China Postdoctoral Science Foundation [2019M662929]
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NiFe(2)O(4)has been regarded as one of the promising candidates for lithium-ion battery (LIB) anode materials due to its high theoretical specific capacity. However, the large volume expansion and pulverization of NiFe(2)O(4)during the charge/discharge process result in severe capacity fading. Herein, heterostructured NiFe2O4-C nanorods have been successfully fabricated by recovering transition metals from simulated electroplating sludge leaching solution. The constructed NiFe2O4-C heterointerface plays a vital role in accommodating volume change, stabilizing the reaction products and providing rapid electron and Li(+)ion transportation ability, resulting in a high and stable Li(+)accommodation performance. The fabricated NiFe2O4-C nanorods demonstrate a high specific capacity (889.9 mA h g(-1)at 100 mA g(-1)), impressive rate capability (861.5, 704.5, 651.4, 579.6 and 502.1 mA h g(-1)at 0.2, 0.6, 1.0, 2.0 and 5.0 A g(-1)) and cycling stability (650.2 mA h g(-1)at 2 A g(-1)after 500 cycles). This work exemplifies a facile and effective approach for the fabrication of high performance LIB electrode materials by recycling metals from electroplating sludge in an application-oriented manner.
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