Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 69, Pages 9990-9993Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc04289g
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Funding
- National Natural Science Foundation of China [61890940, 51903052, 51903051]
- Shanghai Pujiang Project [19PJ1400700]
- MOE Tier 2 grant [MOE2018-T2-2-094]
- NRF Investigatorship [NRF-NRFI05-2019-0005]
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A heterocycloarene derivative (S-Octulene) possessing two sulfur atoms was conveniently synthesized through Bi(OTf)(3)-catalyzed cyclization from a macrocyclic tetramethoxyethenylated precursor. The physical properties ofS-Octuleneand its supramolecular host-guest interaction with C-60 and C-70 were investigated by fluorescence titration and H-1 NMR. The solution-processed organic field-effect transistor (OFET) measurements demonstrated thatS-Octulenebehaved as a p-type semiconductor with a hole mobility exceeding 0.01 cm(2) V-1 s(-1). Our findings pave a new path to design novel heterocycloarenes for the development of host-guest chemistry and organic semiconductors.
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