Journal
INORGANIC CHEMISTRY
Volume 56, Issue 7, Pages 4021-4027Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.6b03134
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Funding
- Polish Ministry of Science and Higher Education within the Iuventus Plus Programme [0370/IP3/2015/73]
- National Science Centre within the Opus 8 research project [DEC-2014/15/B/ST5/04465]
- U.S. Department of Energy, Basic Energy Sciences, Materials Sciences Division [DE-FG02-02ER45999, DE-SC0012582]
- Robert A. Welch Foundation [A-1449]
- Polish Ministry of Science and Higher Education within the Diamentowy Grant Programme [0041/DIA/2015/44]
- European Regional Development Fund in the framework of the Polish Innovation Economy Operational Program [POIG.02.01.00-12-023/08]
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A building block approach has been used to prepare a new family of hexanuclear magnetic molecules Mn4Nb2, Fe4Nb2, and Co4Nb2 of general formula [M-II(tmphen)(2)](4)[Nb-IV(CN)(8)](2)}center dot solv (M = Mn, Fe, Co; tmphen = 3,4,7,8-tetramethyl-1,10-phenanthroline; solv = MeOH and/or H2O). Mn4Nb2 exhibits a magnetocaloric effect at temperatures close to 1.8 K, and Fe4Nb2 undergoes an incomplete gradual spin crossover and a photomagnetic response related to light-induced excited spin state trapping.
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