4.7 Article

Facile formation of agarose hydrogel and electromechanical responses as electro-responsive hydrogel materials in actuator applications

Journal

CARBOHYDRATE POLYMERS
Volume 247, Issue -, Pages -

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.carbpol.2020.116709

Keywords

Agarose; Electro-responsive hydrogel; Electromechanical properties; Electro-induced bending response; Soft actuator

Funding

  1. 100th Anniversary Chulalongkorn University Fund for Doctoral Scholarship
  2. Conductive and Electroactive Polymers Research Unit of Chulalongkorn University (CEAP)
  3. 90th Anniversary of Chulalongkorn University Fund (Ratchadaphiseksomphot Endowment Fund)
  4. Thailand Science Research and Innovation Fund (TSRI)
  5. National Research Council of Thailand (NRCT)

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The agarose hydrogels (AG HyGels) were fabricated by a solvent casting method at various agarose concentrations, resulting in the 3D hydrogel networks via the physical crosslinking from the hydrogen bonding. The actuator performances were investigated at various agarose contents and electric field strengths. For the electromechanical properties, the AG HyGel_12.0 %v/v possessed the highest storage modulus (G') and storage modulus relative response (Delta G'/G'(0)) of 4.48 x 10(6) Pa and 1.07, respectively under applied electric field strength of 800 V/mm due to the electrostriction effect. In the electro-induced bending measurement, the highest deflection distance was obtained from the AG HyGel_2.0 %v/v due to its initial lower rigidity. Relative to other bio based hydrogels, the present AG HyGels are first demonstrated here as electroactive materials showing comparable magnitudes in the electroactive responses, but with the simple fabrication method without toxic ingredients required. Thus, the present AG HyGels are potential material candidates for soft actuator applications.

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