Journal
ELECTROCHEMICAL ENERGY REVIEWS
Volume 3, Issue 3, Pages 541-580Publisher
SPRINGERNATURE
DOI: 10.1007/s41918-020-00070-7
Keywords
Dealloying; Lithium batteries; Nanoporous; Rechargeable; Electrodes
Categories
Funding
- National Key Research and Development Program of China [2019YFA0205700]
- National Natural Science Foundation of China [51602219, 51671145]
- National Science Fund for Distinguished Young Scholars [51825102]
- NSFC [51761165012]
- Macau Science and Technology Fund (FDCT) [002/2017/AFJ]
- Tianjin Municipal Science and Technology Commission [17JCYBJC42000]
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Dealloying has been recognized as a universal strategy to fabricate various functional electrode materials with open networks, nanoscale ligaments, tunable pore sizes and rich surface chemistry, all of which are very attractive characteristics for rechargeable lithium batteries. In particular, lithium ion insertion/extraction in metal anodes is naturally associated with the alloying/dealloying mechanism. The past decade has witnessed rapid growth of this research field with enormous progress. In this review article, we first summarize the recent development and microstructural regulation of dealloyed materials. Next, we focus on the rational design of nanoporous electrodes for rechargeable lithium batteries and related structure-performance correlations. Finally, some critical issues and perspectives are presented to guide the future development directions of such promising technology for high-energy batteries.
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